首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   560篇
  免费   72篇
  国内免费   269篇
安全科学   17篇
废物处理   9篇
环保管理   35篇
综合类   625篇
基础理论   94篇
污染及防治   72篇
评价与监测   16篇
社会与环境   30篇
灾害及防治   3篇
  2024年   6篇
  2023年   19篇
  2022年   40篇
  2021年   37篇
  2020年   43篇
  2019年   53篇
  2018年   41篇
  2017年   36篇
  2016年   38篇
  2015年   44篇
  2014年   39篇
  2013年   59篇
  2012年   48篇
  2011年   49篇
  2010年   36篇
  2009年   40篇
  2008年   33篇
  2007年   20篇
  2006年   34篇
  2005年   24篇
  2004年   21篇
  2003年   13篇
  2002年   18篇
  2001年   12篇
  2000年   22篇
  1999年   17篇
  1998年   19篇
  1997年   7篇
  1996年   5篇
  1995年   9篇
  1994年   5篇
  1993年   4篇
  1992年   1篇
  1991年   2篇
  1990年   2篇
  1989年   1篇
  1987年   1篇
  1984年   1篇
  1982年   1篇
  1979年   1篇
排序方式: 共有901条查询结果,搜索用时 15 毫秒
91.
Studies on the distribution and isotope compositions of fallout Pu are important for source characterization of possible future non-fallout Pu contamination in aquatic environments, and useful for dating of recent sediments to understand the pollution history of environmental contaminants. We present the historical record of atmospheric Pu fallout reconstructed from a sediment core from Lake Hongfeng, China. The Pu activity profile was in agreement with the 137Cs profile. Inventories were 50.7 Bq m(-2) for 239+240Pu and 1586 Bq m(-2) for 137Cs. The average 240Pu/239Pu atom ratio was 0.185+/-0.009, indicating that Pu originated from global stratospheric fallout rather than from direct tropospheric or close-in fallout from the Chinese nuclear testing conducted in the 1970s. Our data suggested that Lake Hongfeng would be an ideal setting for monitoring atmospheric fallout and environmental changes in this region.  相似文献   
92.
溶液中Al3 、Al-F和有机络合态铝(Al-OM的浓度随pH降低而增加,Al3 在总单核铝中所占比例随pH的降低而增加,而Al-F络合物呈相反的变化趋势.土壤中铝的溶解度与土壤中铝氧化物的结晶形态有关,处于较高纬度地区的土壤,由于铝氧化物的结晶形态较差,在相同pH下,其铝的溶解度较大.土壤溶液中有机络合态铝的浓度随温度升高而增加,在pH不变的情况下,土壤中无机铝的溶解量随温度降低而增加.随水土比增加,土壤溶液中Al3 、Al-F络合物和Al-OM浓度减小,但按每kg土计算的铝溶解量随水土比的增加而增加.  相似文献   
93.
INTRODUCTION: Using data from the NASS General Estimates System (GES), the method of induced exposure was used to assess the effects of electronic stability control (ESC) on loss-of-control type crashes for sport utility vehicles. METHOD: Sport utility vehicles were classified into crash types generally associated with loss of control and crash types most likely not associated with loss of control. Vehicles were then compared as to whether ESC technology was present or absent in the vehicles. A generalized additive model was fit to assess the effects of ESC, driver age, and driver gender on the odds of loss of control. In addition, the effects of ESC on roads that were not dry were compared to effects on roads that were dry. RESULTS: Overall, the estimated percentage reduction in the odds of a loss-of-control crash for sport utility vehicles equipped with ESC was 70.3%. Both genders and all age groups showed reduced odds of loss-of-control crashes, but there was no significant difference between males and females. With respect to driver age, the maximum percentage reduction of 73.6% occurred at age 27. The positive effects of ESC on roads that were not dry were significantly greater than on roads that were dry.  相似文献   
94.
In recent years, compound specific isotope analyses (CSIA) have developed into one of the most powerful tools for the quantification of in situ biodegradation of organic contaminants. In this approach, the calculation of the extent of biodegradation of organic contaminants in aquifers is usually based on the Rayleigh equation, and thus neglects physical transport processes such as dispersion that contribute to contaminant dilution in aquifers. Here we combine compound specific isotope analyses with a conservative transport model to study the attenuation of aromatic hydrocarbons at a former gasworks site. The conservative transport model was first used to simulate concentration reductions caused by dilution at wells downgradient of a BTEX source. In a second step, the diluted concentrations, together with the available stable carbon isotope ratios and carbon fractionation factors for benzene, toluene and o-xylene were applied in the Rayleigh equation to quantify the degree of biodegradation at each of those wells. At the investigated site, where other attenuation processes such as sorption and volatilisation were proven to be negligible, the combined approach is recommended for benzene, which represents a compound for which the effect of biodegradation is comparable to or less than the effect of dilution. As demonstrated for toluene and o-xylene, the application of the Rayleigh equation alone is sufficient if dilution can be proved to be insignificant in comparison to biodegradation. The analysis also suggests that the source width and the position of the observation wells relative to the plume center line are significantly related to the degree of dilution.  相似文献   
95.
全新世青藏高原东部西南季风的演变   总被引:3,自引:0,他引:3  
本研究报道一组新的西南季风代用指标,即泥炭中单一种属植物———木里苔草残体纤维素和泥炭混合植物残体纤维素的δ13C时间序列,所记录的青藏高原东部全新世气候变化。两记录表明,该区全新世的下限年龄约11200aBP(14C年龄约9900aBP);从约11200aBP起该区迅速进入湿暖的全新世阶段,季风活动迅速增强;在约10800~5500aBP期间,季风总体保持在强盛状态,但其间有4次突然减弱,气候变干冷;约从5500aBP起季风活动在波动中逐渐减弱,其中有4次减弱最明显。所有这8次气候的突然变化都与北大西洋浮冰事件一一对应。这种密切的相关关系表明,西南季风强度的波动可能是对全球变化,特别是对海洋热盐环流引起的地球南北方气候波动的所谓"跷跷板效应"的响应。  相似文献   
96.
高阶段尾砂胶结充填体力学研究与博弈树配比优化   总被引:4,自引:0,他引:4  
在实验室试验了不同配比尾砂胶结试块强度,在充填采场取样测试了采场充填体强度.结果表明,如果以实验室试验的力学参数为充填配比设计依据,充填体最小设计安全系数为1.6~1.8比较合理.分析高阶段充填体受力,推导了分层充填力学计算公式及安全系数计算方法;根据充填工艺,确定最小充填高度,沿采场高度方向划分配比优化单元,建立了高阶段充填体配比优化设计模型;采用博弈树分析方法,解决了高阶段充填体配比优化问题,并对安庆铜矿5号矿房配比进行了优化.结果显示:与经验设计方法相比,采用本文方法优化充填配比,不仅使高阶段充填体内安全系数分布更趋合理,而且降低了水泥消耗.  相似文献   
97.
安全稳定性是凸轮机构运行的首要要求,从凸轮机构设计入手,在理论上分析了压力角和基圆半径对机构运行稳定性的影响。稳定性的影响因素很多,本文指出压力角和基圆半径的确定,要把理论计算和实际经验结合,确定恰当的参数,提高机构运行的稳定性,可靠性。  相似文献   
98.
三维电极电Fenton氧化法处理染料废水   总被引:1,自引:0,他引:1       下载免费PDF全文
采用三维电极电Fenton氧化法处理实际染料废水,探究了染料废水处理效果的影响因素。实验结果表明:以钌铱镀层钛电极为阳极、不锈钢板为阴极、粉末活性炭为颗粒电极,在粉末活性炭投加量为2.0 g/L、电流密度为0.5 mA/mm2、极板间距为3 cm、pH为2.0、硫酸亚铁投加量为0.50 g/L的最优工艺条件下,反应2 h后COD、TOC、氨氮、色度的去除率达到最大,分别为62.80%、41.15%、42.48%和95.00%;粉末活性炭作为颗粒电极可使染料废水COD去除率提高18个百分点;重复使用10次的处理效果与第2次基本持平。  相似文献   
99.
In the Ohio River (OR), backwater confluence sedimentation dynamics are understudied, however, these river features are expected to be influential on the system’s ecological and economic function when integrated along the river’s length. In the following paper, we test the efficacy of organic and inorganic tracers for sediment fingerprinting in backwater confluences; we use fingerprinting results to evidence sediment dynamics controlling deposition patterns in confluences used for wetland and marina functions; and we quantify the spatial extent of tributary drainages with wetland and marina features in OR confluences. Both organic and inorganic tracers statistically differentiate sediment from stream and river end‐members. Carbon and nitrogen stable isotopes produce greater uncertainty in fingerprinting results than inorganic elemental tracers. Uncertainty analysis of the nonconservative tracer term in the organic matter fingerprinting application estimates an apparent enrichment of the carbon stable isotopes during instream residence, and the nonconservativeness is quantified with a statistical approach unique to the fingerprinting literature. Wetland and marina features in OR confluences impact 42% and 11% of tributary drainage areas, respectively. Sediment dynamics show wetland and marina confluences experience deposition from river backwaters with longitudinally linear and nonlinear patterns, respectively, from sediment sources.  相似文献   
100.
This article is the most recent report of polycyclic aromatic hydrocarbons (PAHs) in the Muar River and Pulau Merambong, Peninsular Malaysia. A total of 16 priority pollutant PAHs in addition to methylphenanthrene among alkylated PAHs were analyzed in surface sediments during May 2013. Total PAHs ranged from 212 to 440 and 151 to 412 ng g?1 dw in sediments from the Muar River and the Pulau Merambong, respectively. The Muar River showed an increasing trend of PAH concentrations, while no previous data exist for the Pulau Merambong. Generally, mixed petrogenic and pyrogenic sources of PAHs with predominance of the latter were detected in the study area. Effective management of oil pollution has caused a drastic decrease in petrogenic sources of PAHs.  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号